RT Journal Article T1 Two-dimensional oligoglycine tectomer adhesives for graphene oxide fiber functionalization A1 Garriga, R. A1 Jurewicz, I. A1 Seyedin, S. A1 Tripathi, M. A1 Pearson, J. R. A1 Cebolla, V. L. A1 Dalton, A. B. A1 Razal, J. M. A1 Munoz, E. K1 In-situ synthesis K1 Gold nanoparticles K1 Carbon nanotube K1 Chitosan K1 Hybrid K1 Chemistry K1 Yarns K1 Silk AB Amino-terminated oligoglycine two-dimensional (2D) peptide self-assemblies (known as tectomers) have a versatile surface chemistry that allows them to interact with a variety of nanomaterials and to act as supramolecular adhesives for surface functionalization. Here, we have exploited the strong hydrogenbond based interaction between tectomers and graphene oxide (GO) to functionalize GO fiber surfaces with different carbon nanomaterials (carbon nanotubes, carbon nanohorns, carbon nanocones, and highly fluorescent nanodiamonds), metal (gold, platinum, iron) nanoparticles, acrylate-based polymer nanoparticles, fluorophores and drugs. The resulting ultrathin coatings exhibit remarkable water resistant properties. This tectomer-mediated fiber decoration strategy allows coating functionalities to be tailored by choosing the appropriate nanomaterials or other molecules. We show that this strategy can be extended to other fibers and fabrics, such as polyurethane/ PEDOT: PSS, poly(methyl methacrylate) and polyester, making it very attractive for a variety of technological and smart textile applications. (C) 2019 Elsevier Ltd. All rights reserved. PB Pergamon-elsevier science ltd SN 0008-6223 YR 2019 FD 2019-06-01 LK https://hdl.handle.net/10668/26567 UL https://hdl.handle.net/10668/26567 LA en DS RISalud RD Apr 17, 2025